Ongoing research is focused on inorganic, random porous materials and incorporates expertise at the interface of chemistry and materials science to develop the next generation of sustainable construction materials. The work incorporates aspects of first principles and continuum scale simulations and integrated experiments, ranging from nano-to-macro scales. Special efforts are devoted toward developing low-clinker factor cements and concretes, reducing the carbon footprint of construction materials, and increasing the service life of civil engineering infrastructure.